Overview of the model system. (IMAGE)

Ultrafast Science

Overview of the model system.

Caption

Overview of the model system. (A) One-dimensional slices of the PESs along the R1 reaction coordinate are shown. The black dashed circle shows the point of degeneracy between the two electronic states. Vertical arrows indicate transitions between the electronic states. Transition A corresponds to an electronic state separation of ≈2.2 eV, and transition B corresponds to an electronic state separation of ≈0.8 eV. (B) Two-dimensional representation of the adiabatic PESs for the electronic states involved in the CI. (C) The population dynamics of the V0 state (blue) and V1 state (red). The time delay axis is referenced with respect to the pump–pulse interaction.

Credit

Ultrafast Science

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